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Quantum transport properties of the topological Dirac semimetal α-Sn
Md Shahin Alam, Alexandr Kazakov, Mujeeb Ahmad, Rajibul Islam, Fei Xue, and Marcin Matusiak
Phys. Rev. B 109, 245135 – Published 26 June 2024
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Abstract
We report on measurements of the electrical resistivity (ρ) and thermoelectric power () in a thin film of strained single-crystalline α-Sn grown by molecular beam epitaxy on an insulating substrate. The temperature () dependence of the resistivity of α-Sn can be divided into two regions: below K ρ() shows metalliclike behavior, while above this temperature, an increasing contribution from thermally excited holes to electrical transport is observed. However, it is still dominated by highly mobile electrons, resulting in a negative sign of the Seebeck coefficient above K. In the presence of the magnetic field () applied along an electric field or thermal gradient, we note negative magnetoresistance or a negative slope of (), respectively. The theoretical prediction for the former (calculated using density functional theory) agrees well with the experiment. However, these characteristics quickly disappear when the magnetic field is deviated from an orientation parallel to the electrical field or the thermal gradient. We indicate that the behavior of the electrical resistivity and thermoelectric power can be explained in terms of the chiral current arising from the topologically nontrivial electronic structure of α-Sn. Its decay at high temperature is a consequence of the decreasing ratio between the intervalley Weyl relaxation time to the Drude scattering time.
- Received 29 February 2024
- Revised 30 April 2024
- Accepted 7 June 2024
DOI:https://doi.org/10.1103/PhysRevB.109.245135
©2024 American Physical Society
Physics Subject Headings (PhySH)
- Research Areas
MagnetotransportTopological materialsTransport phenomena
- Physical Systems
Dirac semimetal
- Techniques
Density functional theoryTransport techniques
Condensed Matter, Materials & Applied Physics
Authors & Affiliations
Md Shahin Alam1,*, Alexandr Kazakov1, Mujeeb Ahmad1, Rajibul Islam2, Fei Xue2, and Marcin Matusiak1,3,†
- 1International Research Centre MagTop, Institute of Physics, Polish Academy of Sciences, Aleja Lotników 32/46, PL-02668 Warsaw, Poland
- 2Department of Physics, University of Alabama at Birmingham, Birmingham, Alabama 35294, USA
- 3Institute of Low Temperature and Structure Research, Polish Academy of Sciences, ulica Okólna 2, 50-422 Wrocław, Poland
- *Contact author: shahin@magtop.ifpan.edu.pl
- †Contact author: m.matusiak@intibs.pl
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Issue
Vol. 109, Iss. 24 — 15 June 2024
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Article part of CHORUS
Accepted manuscript will be available starting26 June 2025.![Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (13) Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (13)](https://i0.wp.com/cdn.journals.aps.org/development/journals/images/author-services-placard.png)
Images
Figure 1
Temperature dependences of the resistivity (ρ) and the thermoelectric power () of 200-nm-thick α-Sn thin film where the current () or thermal gradient () is applied parallel to the axis. Inset shows low-temperature thermoelectric power data.
Figure 2
(a) Normalized magnetoresistance vs magnetic field of α-Sn for selected temperatures when both magnetic field and current are applied parallel to the axis ( || ). Magnetothermopower of α-Sn measured with the configuration of applied thermal gradient and magnetic field parallel to the axis (), (b) at low temperatures, and (c) at high temperatures.
Figure 3
(a) The electronic band structure of α-Sn in the presence of spin-orbit coupling using density functional theory (DFT) over the full Brillouin zone (BZ); the BZ is shown in (c); the closer look along → is shown in (b). (d) The two-dimensional (2D) band structure in the () plane illustrates the position of two Dirac points at (0,0, ). (e) Magnetoresistance at θ = 0° magnetic field orientations, influenced by Fermi surface topology.
Figure 4
(a) Resistivity () in function of magnetic field () of Dirac semimetal α-Sn for selected angles (, where is the angle between and ) at a constant temperature 60 K. (b) Magnetothermopower of α-Sn for selected angles (, where is the angle between and ) at a constant temperature 60 K.
Figure 5
(a) Conductivity () in function of square of magnetic field () of α-Sn for several temperatures. For the sake of clarity, starting from for = 38 K, the curves are successively shifted vertically by each for sake of clarity. (b) Normalized thermopower () of α-Sn for selected temperatures. The dashed line in both panels shows the fit as calculated from Eqs.(2) and (3).
Figure 6
The ratio of intervalley Weyl scattering time to Drude relaxation time (/τ) of the α-Sn sample as a function of temperatures with the current () or thermal gradient () along with the magnetic field applied parallel to the axis.