Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (2024)

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Quantum transport properties of the topological Dirac semimetal α-Sn

Md Shahin Alam, Alexandr Kazakov, Mujeeb Ahmad, Rajibul Islam, Fei Xue, and Marcin Matusiak
Phys. Rev. B 109, 245135 – Published 26 June 2024
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Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (1)

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    Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (2)

    Abstract

    We report on measurements of the electrical resistivity (ρ) and thermoelectric power (S) in a thin film of strained single-crystalline α-Sn grown by molecular beam epitaxy on an insulating substrate. The temperature (T) dependence of the resistivity of α-Sn can be divided into two regions: below T*135 K ρ(T) shows metalliclike behavior, while above this temperature, an increasing contribution from thermally excited holes to electrical transport is observed. However, it is still dominated by highly mobile electrons, resulting in a negative sign of the Seebeck coefficient above T=47 K. In the presence of the magnetic field (B) applied along an electric field or thermal gradient, we note negative magnetoresistance or a negative slope of S(B), respectively. The theoretical prediction for the former (calculated using density functional theory) agrees well with the experiment. However, these characteristics quickly disappear when the magnetic field is deviated from an orientation parallel to the electrical field or the thermal gradient. We indicate that the behavior of the electrical resistivity and thermoelectric power can be explained in terms of the chiral current arising from the topologically nontrivial electronic structure of α-Sn. Its decay at high temperature is a consequence of the decreasing ratio between the intervalley Weyl relaxation time to the Drude scattering time.

    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (3)
    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (4)
    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (5)
    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (6)
    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (7)
    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (8)
    • Received 29 February 2024
    • Revised 30 April 2024
    • Accepted 7 June 2024

    DOI:https://doi.org/10.1103/PhysRevB.109.245135

    ©2024 American Physical Society

    Physics Subject Headings (PhySH)

    1. Research Areas

    MagnetotransportTopological materialsTransport phenomena

    1. Physical Systems

    Dirac semimetal

    1. Techniques

    Density functional theoryTransport techniques

    Condensed Matter, Materials & Applied Physics

    Authors & Affiliations

    Md Shahin Alam1,*, Alexandr Kazakov1, Mujeeb Ahmad1, Rajibul Islam2, Fei Xue2, and Marcin Matusiak1,3,†

    • *Contact author: shahin@magtop.ifpan.edu.pl
    • Contact author: m.matusiak@intibs.pl

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    Vol. 109, Iss. 24 — 15 June 2024

    Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (9)
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    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (14)

      Figure 1

      Temperature dependences of the resistivity (ρ) and the thermoelectric power (S) of 200-nm-thick α-Sn thin film where the current (J) or thermal gradient (T) is applied parallel to the a axis. Inset shows low-temperature thermoelectric power data.

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    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (15)

      Figure 2

      (a) Normalized magnetoresistance vs magnetic field of α-Sn for selected temperatures when both magnetic field and current are applied parallel to the a axis (B || j). Magnetothermopower of α-Sn measured with the configuration of applied thermal gradient and magnetic field parallel to the a axis (T||B), (b) at low temperatures, and (c) at high temperatures.

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    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (16)

      Figure 3

      (a) The electronic band structure of α-Sn in the presence of spin-orbit coupling using density functional theory (DFT) over the full Brillouin zone (BZ); the BZ is shown in (c); the closer look along MΓZ is shown in (b). (d) The two-dimensional (2D) band structure in the (kxkz) plane illustrates the position of two Dirac points at (0,0, ±kz). (e) Magnetoresistance at θ = 0° magnetic field orientations, influenced by Fermi surface topology.

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    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (17)

      Figure 4

      (a) Resistivity (ρxx) in function of magnetic field (B) of Dirac semimetal α-Sn for selected angles (θ, where θ is the angle between j and B) at a constant temperature 60 K. (b) Magnetothermopower [Sxx(B)] of α-Sn for selected angles (θ, where θ is the angle between T and B) at a constant temperature 60 K.

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    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (18)

      Figure 5

      (a) Conductivity (σ) in function of square of magnetic field (B) of α-Sn for several temperatures. For the sake of clarity, starting from σ(B2) for T = 38 K, the curves are successively shifted vertically by 102Ω1cm1 each for sake of clarity. (b) Normalized thermopower S(B) of α-Sn for selected temperatures. The dashed line in both panels shows the fit as calculated from Eqs.(2) and (3).

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    • Quantum transport properties of the topological Dirac semimetal \ensuremath{\alpha}-Sn (19)

      Figure 6

      The ratio of intervalley Weyl scattering time to Drude relaxation time (τi/τ) of the α-Sn sample as a function of temperatures with the current (j) or thermal gradient (T) along with the magnetic field applied parallel to the a axis.

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